Active dipole clusters: From helical motion to fission.

The structure of a finite particle cluster is typically determined by total energy minimization. Here we consider the case where a cluster of soft-sphere dipoles becomes active, i.e., when the individual particles exhibit an additional self-propulsion along their dipole moments. We numerically solve the overdamped equations of motion for soft-sphere dipoles in a solvent. Starting from an initial metastable dipolar cluster, the self-propulsion generates a complex cluster dynamics. The final cluster state has in general a structure widely different to the initial one, the details depend on the model parameters and on the protocol of how the self-propulsion is turned on. The center of mass of the cluster moves on a helical path, the details of which are governed by the initial cluster magnetization. An instantaneous switch to a high self-propulsion leads to fission of the cluster. However, fission does not occur if the self-propulsion is increased slowly to high strengths. Our predictions can be verified through experiments with self-phoretic colloidal Janus particles and for macroscopic self-propelled dipoles in a highly viscous solvent.